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For emulated games, or for PSP games in general? Obviously, the CPU clock speed cap is for battery-saving purposes, but running it at full speed doesn't affect the CPU itself. You'll notice the battery drain, but that's it. Now, if you want 333Mhz overall (versus the normal 222Mhz), then, from what I know, you can only do so in emulators. Unless, of course, you know of another way. Whenever you fully turn the PSP off, everything in the cache is cleared. So that bars anything from being able to consistently OCing the CPU without having to relaunch a program. Not to mention, though, that running the CPU at 333Mhz and then putting it into sleep mode for extended periods of time CAN be damaging (remember, the CPU is still on, just that the amount of energy used is decreased).
Bottom line: No real app to keep the CPU at 333Mhz (not really OCing, just unlocking). Only way of doing so is in emulated games, or homebrew apps that have the option (and even then, the HB apps can't be open if you want to play a retail game).
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